Abstract:
Excessive use of petroleum-based plastic packaging causes severe environmental
pollution due to the low biodegradability, hence the dire need for sustainable
alternatives. Accordingly, large amounts of fruit and vegetable processing wastes
generated in Sri Lanka are rich in cellulose but remain underutilized. In this work, an
attempt was made to develop and evaluate completely biodegradable packaging
material using agricultural waste pulp (AW) in combination with recycled paper waste
(PW) pulp. Peels of carrot, orange, mango, papaye, pineapple, tomato, cabbage, and
passion fruit were chemically and physically treated through bleaching with 10%
NaClO, alkaline digestion using 5% NaOH, ffid neutralization to extract cellulose
fibers, while waste paper was processed to obtain paper pulp. Three formulations were
prepared: Tr (75% AW+Z1VI PW), T, (50% AW+ 50% PW), and Tr (25% AW+ 75Yo
PW), using corn starch as a binder and an Aloe vera, glycerol coating to improve
flexibility, barrier properties, and microbial safety. The experiment was based on a
Completely Randomized Design with replicates, and the developed sheets were
analyzed for differerrt physical, mechanical, chemical, and microbiologica,l properties
such as thickness, hardness, basis weight, density, moisture content, water absorption,
water solubility, pH, color (L*o a*, and b*), cellulose content, biodegradability (soil
burial), and microbial load (TPC and yeast & mold). Significant differences $ < 0.05),
were observed among the treatments. Among these, Tz showed the best overall
performance with the maximum thickness of 91.16 pm, optimal hardness, balanced
density, maximum cellulose content of 59.89%o, and the highest biodegradation rate of
9.31% within 10 days, while LDPE did not degrade considerably. T2 also presented
moderate moisture properties, pH values close to neutrality, better color distribution,
and the lowest microbial load because ofthe application of the Aloe vera-glycerol layer.
The combination of 50To agricultural waste and paper waste presented the optimal
composition regarding tensile strength, biodegradability, water resistance, as well as
the ability to be used as an ecolo gicallysustainable altemativefor packaging made from
petroleum-based plastic.
